Large language models achieve strong performance across diverse tasks, but deployment remains costly because of memory, latency, and energy demands. Structured pruning reduces these costs by removing architectural components, yet its recovery stage is often limited by a mismatch between the recovery module’s representational capacity and the complexity of the removed knowledge. We call this bottleneck the capacity-knowledge asymmetry and propose **OverRep**, an **Over**complete **Rep**arameterization framework for structured LLM pruning. Following the principle of *“train overcomplete, deploy compact”*, OverRep temporarily overparameterizes the recovery module during training to absorb complex knowledge distilled from the original model. After recovery, the overcomplete re-parameterization is algebraically merged into a mathematically equivalent compact module, preserving the pruned model’s inference-time architecture and computational cost. OverRep further introduces an annealed activation that enables nonlinear training dynamics while converging to a linear regime for exact algebraic merging. Across three backbone families, OverRep improves retained reasoning performance over strong recovery baselines by up to 5.5 and 8.4 points at 25% and 50% pruning, respectively, while keeping memory usage and TFLOPs comparable to existing recovery methods. Our code is available at https://github.com/mmai-laboratory/OverRep

In this paper, we introduce layer-wise curriculum learning aimed at efficient LLM compression. The proposed method facilitates the transfer of knowledge from the teacher to student model, utilizing a curriculum learning approach that begins with easier optimization tasks and progressively tackles much harder ones. In order to adopt the layer-wise learning in LLM compression, we partition the whole model into multiple segments consisting of layers, thereby enabling more computationally efficient knowledge transfer of LLMs. Based on the theoretical evidence of cumulative error phenomenon, layer-wise curriculum learning accelerates convergence while stabilizing the knowledge transfer process. In addition, we present a feature caching method with a multi-threading strategy to efficiently address feature misalignment across layers, maximizing GPU utilization. Consequently, our method exhibits advanced model compression performance, as well as high computational efficiency in terms of minimized memory usage and short training hours. Experiments on multiple datasets show that the proposed method achieves state-of-the-art performance while reducing GPU memory usage and training hours by more than 50% on BERT and GPT-2. Moreover, it outperforms the other pruning methods on LLaMA-family and Qwen under the same training hours, with a lower GPU memory footprint. Upon acceptance, we will publicly release the code to support the reproducibility of our results.